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Lead Halide Perovskites: Challenges and Opportunities in Advanced Synthesis and Spectroscopy

TitleLead Halide Perovskites: Challenges and Opportunities in Advanced Synthesis and Spectroscopy
Publication TypeJournal Article
Year of Publication2017
AuthorsRosales, BA, Hanrahan, MP, Boote, BW, Rossini, AJ, Smith, EA, Vela, J
JournalAcs Energy Letters
Volume2
Pagination906-914
Date Published04
Type of ArticleArticle
ISBN Number2380-8195
Accession NumberWOS:000399636600027
Keywordscation, ch3nh3pbi3, chemistry, Electrochemistry, fuels, luminescence, magnetic-resonance, Materials Science, nanocrystals, nmr, organometal trihalide perovskite, Other Topics, solar-cells, stability, Technology -, wide color gamut
Abstract

Pb solid-state nuclear magnetic resonance and single-particle photoluminescence spectroscopies show that the structure and composition of mixed-halide and likely other hybrid lead perovskites are much more complex than previously thought and are highly dependent on their synthesis. While a majority of reports in the area focus on the construction of photovoltaic devices, this Perspective focuses instead on achieving a better understanding of the fundamental chemistry and photophysics of these materials, because this will aid not only in constructing improved devices but also in generating new uses for these unique materials.

DOI10.1021/acsenergylett.6b00674
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Short TitleACS Energy Lett.
Alternate JournalACS Energy Lett.