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Femtosecond switching of magnetism via strongly correlated spin-charge quantum excitations

TitleFemtosecond switching of magnetism via strongly correlated spin-charge quantum excitations
Publication TypeJournal Article
Year of Publication2013
AuthorsLi, TQ, Patz, A, Mouchliadis, L, Yan, JQ, Lograsso, TA, Perakis, IE, Wang, JG
JournalNature
Volume496
Pagination69-73
Date Published04
Type of ArticleArticle
ISBN Number0028-0836
Accession NumberWOS:000316993400026
Keywordsdensity-wave, manganite, order, phase-separation, pulses, state, transition-metal oxides, ultrafast
Abstract

breaking the delicate balance between competing phases of correlated materials: for example, manganites exhibiting colossal magneto-resistance suitable for applications(3,4). Here we show femtosecond (10(-15) seconds) photo-induced switching from anti-ferromagnetic to ferromagnetic ordering in Pr0.7Ca0.3MnO3, by observing the establishment (within about 120 femtoseconds) of a huge temperature-dependent magnetization with photo-excitation threshold behaviour absent in the optical reflectivity. The development of ferromagnetic correlations during the femtosecond laser pulse reveals an initial quantum coherent regime of magnetism, distinguished from the picosecond (10(-12) seconds) lattice-heating regime characterized by phase separation without threshold behaviour(5,6). Our simulations reproduce the nonlinear femtosecond spin generation and underpin fast quantum spin-flip fluctuations correlated with coherent superpositions of electronic states to initiate local ferromagnetic correlations. These results merge two fields, femtosecond magnetism in metals and band insulators(1,7-9), and non-equilibrium phase transitions of strongly correlated electrons(10-17), in which local interactions exceeding the kinetic energy produce a complex balance of competing orders.

DOI10.1038/nature11934
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